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TABLE 4.23. CAESIUM-137 IN THE BOTTOM SEDIMENTS OF THE DNIEPER RESERVOIRS (JANUARY 1995)

Reservoir

Inventory (TBq)

Averaged density of contamination (kBq/m2)

 

 

 

 

 

Kiev

80

± 17

86

± 6

Kanev

18

± 3

31

± 25

Kremenchug

26

± 3

13

± 1

Dniprodzerzhinsk

4.3

± 0.4

7.4

± 0.7

Dnieper

2.2

± 0.7

5.6

± 1.9

Kakhovka

6.8

± 0.7

3.1

± 0.4

Total in cascade

136

± 26

 

 

 

 

 

 

Table 4.23 shows the inventory of 137Cs in the bottom sediments of the Dnieper reservoirs and the averaged densities of the bottom contamination of each reservoir as of January 1995.

As noted above, the mapping of the bottom sediment contamination with 90Sr was problematic. Owing to the low sorption of 90Sr on to solid particles, no regularities in its spatial distribution on the bottom of the reservoirs were discovered. However, where there is an accumulation of shells of molluscs and other carbonate deposits on the bottom, there are higher levels of 90Sr. It is not excluded that the strong fixation of 90Sr in the carbonate structure of folds is one of the main factors of irretrievable removal of this radionuclide from the water column on to the bottom.

At present, the contaminated bottom sediments in the reservoirs do not influence significantly the secondary radioactive contamination of the water and aquatic organisms. In all places the deposition of cleaner sediments over the more contaminated ones is observed. Thus the general rule for exploitation of the reservoirs (mainly Kiev) is to minimize scooping and mechanical operations at the places with increased bottom contamination. The natural processes of self-cleaning are working in all the reservoirs. As a consequence, there is a gradual reduction in the radionuclide levels in fish and other aquatic species living in the reservoirs.

Results of modelling of the sediment redistribution following a major flood are given in Section 9.3.6.

4.8. CONCLUSIONS

(a)The levels of 137Cs and 90Sr in flowing rivers are now well below the permissible levels set

by the national authorities and below internationally acceptable levels for drinking water.

(b)Surface water runoff from watersheds and floodplains contaminated with 90Sr remains the major contributor to contamination of the Dnieper reservoirs. The main sources contributing to radionuclide releases into the Dnieper cascade are located within the CEZ. The water remedial actions carried out during recent years (1993–2000) significantly reduced actual and potential fluxes into the river.

(c)Almost all the 137Cs washed out of contaminated areas is immobilized in bottom sediments within the reservoirs of the Dnieper River. The impact of these sediments is low and will decline further with decay and further deposition of sediments on top of the contaminated sediments. The overall strategy should be to leave these sediments as is and avoid processes that will lead to their resuspension.

(d)Identification of the main sources within the Chernobyl zone shows that the heavily contaminated floodplain areas still remain the main source for releases. The waste disposal sites in the flood prone areas are of secondary priority for possible remedial actions.

(e)Monitoring systems have been developed for the river systems and are important inputs to the decision making process on possible further water protection measures in the Chernobyl area.

(f)Monitoring data are collected by various agencies for different purposes; different methodologies are used, some of which are outdated. There needs to be harmonization of results between the various organizations engaged in monitoring.

(g)Mathematical models have been developed to describe the wash-off of radioactivity from

61

contaminated land. These models can be used to predict the discharge of radioactivity into rivers and reservoirs from knowledge of the rainfall distribution.

(h)Only a small fraction of the radioactivity deposited on ground via fallout has entered the Dnieper River system, and most of the 137Cs and 90Sr will decay in the ground.

(i)Levels of 137Cs in the lower sections of the

Dnieper River have returned to preChernobyl accident levels. Strontium-90 is more persistent because it does not adsorb as readily on to sediments.

(j)Lakes with no regular inflows and outflows still present a radiological problem that will continue for some time. There is a need for improved understanding of processes occurring within lakes, especially transfer to fish.

(k)Transboundary movement of radionuclides from the Chernobyl accident was greatest prior to 1990. The annual flows of 137Cs across national borders have continued to decline steadily, whereas those of 90Sr continue to fluctuate, depending on the extent of flooding of contaminated land (especially the floodplain area of the CEZ). Currently, the annual flow of 137Cs into the Black Sea is negligible, whereas 1–8 TBq of 90Sr reaches the Black Sea.

(l)There is a need for improved understanding of the 90Sr inventory in sediments and 90Sr fixation processes. Strontium-90 becomes more important with time because of its greater mobility.

(m)The large database developed by SPA Typhoon, the UHMI and the RCREM is very useful in understanding and interpreting data, and should be maintained. Ideally it should be expanded to include aquatic species data and data from the lower parts of the Dnieper River.

REFERENCES TO SECTION 4

[4.1] UNITED NATIONS, Sources and Effects of Ionizing Radiation (Report to the General Assembly), Annex J: Exposures and Effects of the Chernobyl Accident, United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR), UN, New York (2000).

[4.2] DE CORT, M., TSATUROV, Y., Atlas of Caesium Deposition on Europe after the Chernobyl Nuclear Power Plant Accident, Final Report of Joint Study Project No. 6, Rep. 16542, Office for Official Publications of the European Communities, Luxembourg (1996).

[4.3] DE CORT, M., Atlas of Caesium Deposition on Europe after the Chernobyl Accident, Rep. 16733, Office for Official Publications of the European Communities, Luxembourg (1998).

[4.4] DE CORT, M., Atlas of Caesium Deposition on Europe after the Chernobyl Accident, Rep. 16733, Office for Official Publications of the European Communities, Luxembourg (2001) CD-ROM.

[4.5] Atlas of Radioactive Contamination of European Part of Russia, Belarus and Ukraine, Federal Service of Geodesy and Cartography of Russia, Moscow (1998).

[4.6] KONOPLEV, A.V., DEVILLE-CAVELIN, G., VOITSEKHOVICH, O.V., ZHUKOVA, O.M., Transfer of Chernobyl 137Cs and 90Sr by surface runoff, Radioprotection-Colloques 37 C1 (2002) 315–318.

[4.7] KANIVETS, V., Main tendencies in the Dnieper water system radioactive contamination during the period after the Chernobyl accident, Visnik Agro. Nauki N-4 (1996) 40–56 (in Russian).

[4.8] MAKHONKO, K.P. (Ed.), Instructions for Hydrometeorological Stations and Posts, Issue 12, Monitoring of Radioactive Contamination of the Environment, Hydrometeoizdat, Leningrad (1982) (in Russian).

[4.9] MAKHONKO, K.P. (Ed.), Manual on Organization of Monitoring of the State of the Environment in the Area of NPP, Hydrometeoizdat, St. Petersburg (1990) (in Russian).

[4.10] NIKITIN, A.I. (Ed.), Manual on Control of Radioactive Contamination of Water Bodies, SPA Typhoon, Obninsk (1996) (in Russian).

[4.11] NIKITIN, A.I. (Ed.), Manual on Control of Tritium Content in Water Bodies, SPA Typhoon, Obninsk (1996) (in Russian).

[4.12] VOITSEKHOVITCH, O.V., KANIVETS, V.V., Manual on Carrying out Observations of Radioactive Pollution of the Environment, Ukrainian Hydrometeorological Institute, Kiev (2001) (in Ukrainian).

[4.13] UNITED NATIONS DEVELOPMENT PROGRAMME, Water Quality Evaluation and Prediction in Areas Affected by the Chernobyl Accident (Bryanskaya Oblast), Rep. RUS/95/004, UNDP, Moscow (2001).

[4.14] DEVILLE-CAVELIN, G., BIESOLD, H., BRUN-YABA, C., CHABANYUK, V., The consequences of the Chernobyl accident: First results in the radioecology project of the FrenchGerman initiative, Radioprotection-Colloques 37 C1 (2002) 1043–1048.

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[4.15] KARAUSHEV, A.V., Problems of Dynamics of

Natural Water Flows, Hydrometeoizdat,

Leningrad (1960) (in Russian).

[4.16] VELIKANOV, M.A., Dynamics of Channel

Flows, Hydrometeoizdat, Leningrad (1949) (in

Russian).

[4.17] VAKULOVSKY, S.M. (Ed.), Guidelines on Determination of Radioactive Contamination of Water Bodies, Hydrometeoizdat, Leningrad (1986) (in Russian).

[4.18] Instructions and Guidelines on Evaluation of the Radiation Situation in the Contaminated Territory, Goscomhydromet, Moscow (1989) (in Russian).

[4.19] KANIVETS, V., et al., Results of determinations of 137Cs in water by different laboratories in the measuring section Dnieper–Vyshgorod, unpublished data.

[4.20] VOITSEKHOVITCH, O.V., KANIVETS, V.V., LAPTEV, G.V., Analyses of the Dnieper aquatic system radioactive contamination since five years passed since the accident, Proc. Ukrainian Hydrometeorological Inst. 245 (1993) 106–125 (in Russian).

[4.21] PAVLOTSKAYA, F.I., Migration of Radioactive Products of Global Fallout in Soils, Atomizdat, Moscow (1974) (in Russian).

[4.22] OSIPOV, V.B., Physical and Chemical Behavior of 137Cs and 90Sr and their Stable Isotopes in Soils of Different Ecosystems in Bryansk Region in the Chernobyl Accident Area, PhD thesis, Russian Institute of Agricultural Radiology and Radioecology, Obninsk (1996) (in Russian).

[4.23] BULGAKOV, A.A., KONOPLEV, A.V., “Basic transformation processes of chemical species in soil and bottom sediments”, Modelling and Study of the Mechanisms of the Transfer of Radioactive Material from Terrestrial Ecosystems to and in Water Bodies Around Chernobyl, Final Report (SANSONE, U., VOITSEKHOVICH, O., Eds), Office for Official Publications of the European Communities, Luxembourg (1996) 122–135.

[4.24] KONOPLEV, A.V., et al., “Modelling radiocaesium bioavailability in forest soils”, Contaminated Forests: Recent Developments in Risk Identification and Future Perspectives (LINKOV, I., SHELL, W.R., Eds), Kluwer, Dordrecht (1999) 217–230.

[4.25] SHEVCHOUK, V.E. (Ed.), 15 Years After the Chernobyl Catastrophe: Consequences in the Republic of Belarus and their Overcoming, National Report, Committee on the Problems of the Consequences of the Accident at the Chernobyl NPP, Minsk (2001).

[4.26] KUDELSKY, A.V., SMITH, J.T., ZHUKOVA, O.M., MATVEENKO, I.I., PINCHUK, T.M., The role of river runoff in natural 137Cs decontamination of contaminated areas, J. Rep. NASB 42 (1998) 90–94 (in Russian).

[4.27] MINISTRY OF PUBLIC HEALTH OF THE REPUBLIC OF BELARUS, Republican Permissible Levels of Cesium-137 and Strontium-90 Content in Food Products and Drinking Water, Rep. RPL-99, Ministry of Public Health of the Republic of Belarus, Minsk (1999).

[4.28] VAKULOVSKIY, S.M., et al., “Dynamic of radioactive contamination of rivers of Ukraine, Russia and Belarus due to the accident at the Chernobyl NPP”, Proc. 1st All-Union Conf. on Radiation Aspects of the Chernobyl Accident (IZRAEL, Y.A., Ed.), Hydrometeoizdat, St. Petersburg (1993) 324–331 (in Russian).

[4.29] Water Resources and Water Budget in the Territory of the Soviet Union, Hydrometeoizdat, Leningrad (1967) (in Russian).

[4.30] AQUASCOPE, Final Report: Aquifers and Surface Waters in the Chernobyl Area: Observations and Predictive Evaluation, Project IC15 CT98-0205, Centre for Ecology and Hydrology, Grange-over-Sands, UK (2002).

[4.31] KONOPLEV, A.V., et al., Study of 137Cs and 90Sr behavior in lakes Svyatoe and Kozhanovskoe, Bryansk region, Meteorologiyai Gidrologiya 11 (1998) 45–53 (in Russian).

[4.32] KASHPAROV, V., et. al., Contamination of 30 km Chernobyl exclusion zone, Radiochem. 42 (2001) 550–559 (in Russian).

[4.33] ANTROPOV, V.M., et al., Review and analysis of solid long-lived and high level radioactive waste arising at the Chernobyl nuclear power plant and the restricted zone, DG Environment Project No. B7-5350/99/51983/MAR/C2, Office for Official Publications of the European Communities, Luxembourg (2001) 370.

[4.34] Report on the Study Development of PVLRO Conservation Projects Within the 30-km Exclusion Zone, Phase 17, Assessment of Disposal Safety in PVLRO Kompleksny and Evaluation of the Environmental Impact, Contract No. 247-/96, Zhovti Vody (1996) (in Ukrainian).

[4.35] PANASYUK, N.I., et al., Assessment of the Radiological Contamination of the Geosphere and Calculation of the Radwaste Quantities Localised in the Technogenic Soils and Adjacent to the Unit Shelter, ISTC Shelter Preprint 99-2, ISTC, Chernobyl (1999) (in Ukrainian).

[4.36] BUGAI, D., DJEPO, S., SKALSKY, A., “Prediction of radionuclide migration in geological media, risk assessment and principles of water remedial actions related to groundwater radioactive contamination in the Chernobyl exclusion zone”, Radiogeoecology of the Water Bodies at the Chernobyl Accident Affected Areas, Vol. 2 (VOITSEKHOVITCH, O., Ed.) Chernobylinterinform, Kiev (1998) 218–252.

[4.37] BULGAKOV, A.A., et al., Modelling the longterm dynamics of radiocaesium in closed lakes, J. Environ. Radioact. 61 (2002) 41–53.

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[4.38] BULGAKOV, A.A., KONOPLEV, A.V., KANIVETS, V.V., VOITSEKHOVICH, O.V., Modelling the long-term dynamics of radionuclides in rivers, Radioprotection-Colloques 37 C1 (2002) 649–654.

[4.39] TSATUROV, Y.S., et al., Levels and dynamics of the contamination with the Chernobyl-origin radionuclides of surface water and catchment territory in the western areas of the Bryansk region, Geol. Bull. Cent. Reg. Russia, No. 2 (2001) 5–9.

[4.40] NOVITSKY, M.A., NIKITIN, A.I., Prediction of radioactive contamination of water bodies after the Chernobyl accident, Radiat. Prot. Dosim. 64 (1996) 29–32.

[4.41] ZHUKOVA, O., SHIRYAEVA, N., SHAGALOVA, E., “Water migration of Chernobyl radionuclides in rivers of Belarus”, Radioprotec- tion-Colloques 37 C1 (2002) 723–728.

[4.42] VAKULOVSKY, S.M., et al., Cs-137 and Sr-90 contamination of water bodies in the areas affected by releases from the Chernobyl nuclear power plant accident: An overview, J. Environ. Radioact. 23 (1994) 103–122.

[4.43] NOVIKOV, B.I., TIMCHENKO, V.M., Hydrological conditions of radionuclide migration through the Dnieper’s reservoir, J. Water Resour. N-1 (1992) 95–102.

[4.44] VOITSEKHOVITCH, O., LAPTEV, G., KANIVETS, V., Radioactive contamination of the water bodies in the Chernobyl exclusion zone, Bull. Ecol. Status Chernobyl Exclusion Zone, No. 6 (1996) 37–44.

[4.45] BOCHKOV, L.P., VAKULOVSKY, S.M., NIKITIN, A.I., TERTYSHNIK, E.G., CHUMICHEV, V.B., Activity concentration of 137Cs in terrestrial surface waters, Meteorologiyai Gidrologiya 8 (1983) 79–83.

[4.46] VOITSEKHOVITCH, O.V., Water Quality Management at the Area Affected by the Chernobyl Accident, Ukrainian Hydrometeorological Institute, Kiev (2001) (in Russian).

[4.47] OGORODNIKOV, V., KANIVETS, V., Bottom sediment of the Kiev Reservoir, Proc. Ukrainian Hydrometeorological Institute, No. 245 (1994) 180–194.

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